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The Features of Localized Plasticity Autowaves in Solids

Abstract

The localized plastic deformation and the law-like regularities underlying its development in solids are considered. The characteristic features of localized plasticity are analyzed for a wide range of materials. Thus a correlation is established between the products of scales and of process rates obtained for the elastic and plastic deformation. It is a favorable ground for hypothesizing causal links between the elastic and plastic deformation by introducing an elastic-plastic invariant, which is the master equation of the autowave plasticity model being developed. Localized plasticity phenomena are proposed to be addressed in the frame of autowave and quasi-particle approach.

Keywords:
Elasticity; plasticity; localization; crystal lattice; self-organization; autowave; propagation rate


1. Introduction

During recent decades we have focused on the macro-scale development of plastic flow. The results are presented in papers 11 Zuev LB. Wave phenomena in low-rate plastic flow of solids. Annalen der Physik. 2001;10(11-12):965-984.

2 Zuev LB. On the waves of plastic flow localization in pure metals and alloys. Annalen der Physik. 2007;16(4):286-310.
-33 Zuev LB. Autowave mechanics of plastic flow in solids. Physics of Wave Phenomena. 2012;20(3):166-173. and in the monograph 44 Zuev LB, Barannikova SA. Plastic Flow Localization Viewed as an Auto-Wave Process Generated in Deforming Metals. Solid State Phenomena. 2011;172-174:1279-1283.. We have gradually come to accept that the plastic flow behavior has a characteristic attribute: the deforming medium would spontaneously separate into actively deforming layers alternating with inactive non-deformed layers (Fig. 1). As a result, an intricate arrangement of localized plas ticity patterns would emerge and vary in space and with time. The patterns have been correlated with the flow stages on the stress-strain curves, σ(ε), plotted for the test samples. The available experimental evidence suggests that the patterns in question have space scales ~10-2 m and characteristic times ~102…103 s. The latter two values are virtually unaffected by the kind of material and only slight ly so, by the loading conditions.

Figure 1
Plastic flow localization in the deformed single γ-Fe crystal (a) macrophotograph and (b) series of localized plasticity patterns observed for different times (dark and light bands correspond to active and passive material volumes, respectively)

The stratification of the plastically deforming medium (localization of deformation) is equivalent to the structure formation in the same; hence, this is actually related to the medium’s self-orga niza tion 55 Seeger A, Frank W. Structure Formation by Dissipative Processes in Crystals with High Defect Densities. In: Kubin LP, Martin G, eds. Non-Linear Phenomena in Materials Science. Zurich: Trans Tech Publications; 1987. p. 125-138.,66 Haken H. Information and Self-Organization. A Macroscopic Approach to Complex Systems. 3rd ed. Berlin Heidelberg: Springer-Verlag; 2006.. Our understanding of this fact offers a clearer view of the nature of plasticity. Thus the author is responsible for much of the work on the patterns in question and for identifying them as 'localized plastic flow autowaves'77 Zuev LB. Autowave processes of the localization of plastic flow in active media subjected to deformation. Physics of Metals and Metallography. 2017;118(8):810-819.. The autowave generation is known to involve a decrease in the entropy of the deforming medium 88 Zuev LB. Entropy of localized plastic strain waves. Technical Physics Letters. 2005;31(2):89-90., which counts in favor of the self-organization concept. The autowave length, λ, and the time period, T, have been determined experimentally for similar processes; the values obtained are generally in the range 0.5·10-2λ≤2·10-2m and 102T≤103 s. At about the same time, the theory of solitary plastic waves was put forward for an explanation of plastic flow 99 Hähner P. Theory of solitary plastic waves. Part I: Lüders bands in polycrystals. Applied Physics A. 1994;58(1):41-58.. Here reference should be made to the conceptual representation of other workers 1010 Ananthakrishna G, Valsakumar MC. Repeated yield drop phenomenon: a temporal dissipative structure. Journal of Physics D: Applied Physics. 1982;15(12):L171.,1111 Glazoff MV, Barlat F, Weiland H. Continuum physics of phase and defect microstructures: bridging the gap between physical metallurgy and plasticity of aluminum alloys. International Journal of Plasticity. 2004;20(3):363-402.,1212 Aifantis EC. Gradient plasticity. In: Lemaitre J, ed. Handbook of Materials Behavior Models. New York: Academic Press; 2001. p. 281-307., concerning the nature of periodic processes involved in the plastic deformation. Today the autowave model is substantiated by abundant theoretical and experimental evidence 1212 Aifantis EC. Gradient plasticity. In: Lemaitre J, ed. Handbook of Materials Behavior Models. New York: Academic Press; 2001. p. 281-307.

13 Aifantis EC. On the gradient approach - Relation to Eringen’s nonlocal theory. International Journal of Engineering Science. 2011;49(12):1367-1377.

14 Aifantis EC. Gradient material mechanics: Perspectives and Prospects. Acta Mechanica. 2014;225(4-5):999-1012.

15 Acharia A, Beaudoin A, Miller R. New Perspectives in Plasticity Theory. Dislocation Nucleation, Waves, and Partial Continuity of Plastic Strain Rate. Mathematics and Mechanics of Solids. 2008;13(3-4):292-315.

16 Fressengeas C, Beaudoin AJ, Entemeyer D, Lebedkina T, Lebyodkin M, Taupin V. Dislocation transport and intermittency in the plasticity of crystalline solids. Physical Review B. 2009;79(1):014108.
-1717 Lebyodkin MA, Kobelev NP, Bougherira Y, Entemeyer D, Fressengeas C, Gornakov VS, et al. On the similarity of plastic flow processes during smooth and jerky flow: Statistical analysis. Acta Materialia. 2012;60(9):3729-3740.. It is therefore claimed herein that the auto wave approach has presently received support among scientists.

2. Methods and Materials

The experimental studies of autowave processes of plastic flow were done with the aid of double-exposure speckle photogra phy (Fig. 2 a); due to the stepwise stressing, the method was adapted to high plastic deformation 44 Zuev LB, Barannikova SA. Plastic Flow Localization Viewed as an Auto-Wave Process Generated in Deforming Metals. Solid State Phenomena. 2011;172-174:1279-1283.. The application of the method enables reconstruction of the displacement vector field for the flat sample, i.e.|r(x,y)|>>χ (here χ is the inter pla nar spacing). Using specially developed software, plastic distortion tensor components were calculated for different times and different points on the sample surface (Fig. 2 b). To obtain a generalizable set of data, the experiments were done for a variety of materials having dissimilar nature, which also differed in structure as well as in physical and mechanical properties. The range of studied materials included pure metals and alloys, alkali halide crystals and some rocks 33 Zuev LB. Autowave mechanics of plastic flow in solids. Physics of Wave Phenomena. 2012;20(3):166-173.,44 Zuev LB, Barannikova SA. Plastic Flow Localization Viewed as an Auto-Wave Process Generated in Deforming Metals. Solid State Phenomena. 2011;172-174:1279-1283.. The metals and alloys had FCC, BCC, HCP or tetragonal lattice; these were in single-crystal or polycrystalline state, polycrystalline metals and alloys differing in grain size. We will discuss herein the general regularities of localized plasticity observed for all studied materials.

Figure 2
Localized plasticity in metals (a) - ALMEC-tv measuring system installed on an Instron-1185 testing machine; (b) - distribution of active and passive zones of strain localization; (c) - plastic flow curve and X -t diagram

Autowave processes are likely to originate in the so-called active medium with energy sources distributed throughout its volume 66 Haken H. Information and Self-Organization. A Macroscopic Approach to Complex Systems. 3rd ed. Berlin Heidelberg: Springer-Verlag; 2006.,1818 Dodd RK, Eilbeck JC, Gibbon JD, Morris HC. Solitons and Nonlinear Wave Equations. London: Academic Press; 1982.,1919 Scott A. Nonlinear Science - Emergence and Dynamics of Coherent Structures. New Yok: Oxford University Press; 2003.. The elastic stress fields in the vicinity of stress concentrators play the role of energy sources; hence, the deforming medium meets the condition for autowave generation. An analysis of plastic flow should be based on space-time nonlinear kinetics relations derived for strains and stresses suitable for descriptions of response to loading of a nonlinear deforming medium. The derivation of such relations is considered herein. Moreover, a new universal approach to the phenomenon of solids plasticity is introduced in the form of logical implication. The aim of the given paper is an attempt at revealing the major regularities of the plastic flow by generalization of the diverse database, which would enable elaboration of a persuasive theory of this multivariate phenomenon.

3. The autowave nature of plastic deformation and the elastic-plastic invariant

To gain an insight into the nature of localized plastic deformation, the regular features of its development have to be assessed on the base of qualitative data. The regularities exhibited by the localized plastic flow behavior have been determined with the maximal accuracy for the easy glide and linear work hardening stages. In these cases, the localization patterns comprise a set of localized plasticity nuclei having space and time periods, i.e. autowave length, λ, and characteristic time, T, respectively (Fig. 2 C); hence, the autowave propagation rate, 10-5≤Vaw=dλ/dT≤ 10-4 m/s.

Next Fig. 3 a-c shows the experimentally obtained data characterizing the localized plastic flow autowaves.

Figure 3
Distinctive features of localized plasticity autowaves (а) work hardening coefficient dependence of autowave rate; (b) dispersion relation; (c) grain size dependence of autowave length

3.1 Distinctive features of localized plasticity autowaves

It is found that the autowave rate depends on a dimensionless characteristic of the plastic flow process, i.e. θ=E-1·dσ/dε (here E is the elastic modulus). This dependence has the form

(1) V aw = V 0 + Ξ / θ θ 1 ,

where V0 and Ξ are constants, which differ for the easy glide and linear work hardening stages. (Fig. 3 a).

It should be emphasized that the autowaves observed for the latter two stages are described by the following quadratic dispersion relation (Fig. 3 b),

(2) ω k = ω 0 ± α k k 0 2 ,

where ω=2π/T is frequency; k=2π/λ is wave number and ω0, k0 and α are constants. The mi nus and plus signs correspond to the easy glide and linear work hardening stages, respectively. By substituting ω=ω0·ῶ and k=k0±k˜/α/ω0 into Eq. (2), it is easily reduced to the form ω˜=1±k˜2 (here ῶ and k˜ are dimensionless frequency and wave number, respectively).

The grain size dependence of autowave length, λ(δ), is obtained experimentally for the linear work hardening stage in aluminum (Fig. 3 c). It is described by the logistic function 1919 Scott A. Nonlinear Science - Emergence and Dynamics of Coherent Structures. New Yok: Oxford University Press; 2003. as

(3) λ δ = λ 0 + a 1 / a 2 1 + C exp a 1 δ ,

where λ0, a1 and a2 are empirical constants and C is an integration constant. Function (3) is the solution of the differential equation dλ=a1λa2λ2·dδ 1919 Scott A. Nonlinear Science - Emergence and Dynamics of Coherent Structures. New Yok: Oxford University Press; 2003.. Experimental data analysis suggests that the autowave length depends weakly on the grain size. Thus an increase in the value δ from 10-5 to 10-2 m would cause the value λ to increase from ~6∙10-3 m to ~1.6∙10-2m.

3.2 Introduction of elastic-plastic invariant

At first glance it would seem that Eqs. (1), (2) and (3) are not interrelated; however, we are going to take a good look at these relationships to find out what relation binds them. With this aim in view, quantitative data processing of deformation patterns was performed for studied materials. It has been found that the auto wave characteristics, λ and Vaw, taken together with the spacing, X, and the transverse elastic wave rate, Vt, make up the following ratio (see Table 1)

(4) λ · V aw χ · V t λ χ . V aw V t = const = Z ̂ .

Table 1
Database for introducing elastic-plastic invariant (4).

The calculated data suggest that the average quantity Ẑ=2/3±1/4. Equation (4) is called 'elastic-plastic invariant' by virtue of the fact that it relates the characteristics of elastic waves, X and Vt, to the characteristics of localized plastic flow autowaves, λ and Vaw. The elastic waves are involved in the elastic stress redistribution by the deformation, while the localized plasticity autowaves are in point of fact deformation pattern evolution. Hence, Eq. (4) relates the above two types of processes. This reasoning may play a strategic role in envisaging new conceptual representations of the nature of localized plastic deformation. As is shown in Fig. 4, invariant (4) possesses universality: it is valid for the autowaves pro pa gating at the easy glide and linear stages of work hardening as well as for the motion of individual dislocations 2020 Gillis PP, Gilman JJ. Dynamical Dislocation Theory of Crystal Plasticity. II. Easy Glide and Strain Hardening. Journal of Applied Physics. 1965;36(11):3380-3386..

Figure 4
The meaning of the elastic-plastic invariant • elastic deformation stage; ■ linear work hardening tage; ▲easy glide stage; ♦ individual dislocation motion

In view of Vt2X2ωD2E/ρ (here ωD is the De bye frequency; ρ, material density; E≈X-1∙d2W/du2, elastic modulus; u<<X, displacement and W(u), lattice po tential function 2121 Newnham RE. Properties of Materials - Anisotrophy, Simmetry, Structure. New York: Oxford University Press; 2005.), invariant (4) is rearranged as

(5) V aw λ Z ̂ V t 2 ω D Z ̂ . d 2 W / du 2 ω D χ ρ Z ̂ d 2 W / du 2 ξ 1 ,

where the value ζ1=(ωDX)ρ=Vtρ is the medium's specific acoustic resistance 2222 Lüthi B. Physical Acoustics in the Solid State. Berlin: Springer; 2007..

3.3 Consequences of the elastic-plastic invariant

Eqs. (1) - (3) can be derived from Eq. (4), which suggests that the elastic-plastic invariant plays an important role in the development of autowave concept of localized plasticity.

First, Eq. (4) is differentiated with respect to deformation, ε, as

(6) λ dV aw d ε + V aw d λ d ε = Z ̂ · χ dV t d ε + Z ̂ · V t d χ d ε ·

By writing the above expression with respect to Vaw, we obtain

(7) V aw = d λ d ε 1 Z ̂ · χ dV t d ε + Z ̂ · V t d χ d ε λ dV aw d ε ·

The value X is unaffected by the deformation; hence, Ẑ∙Vt∙dX/dε=0. Consequently,

(8) V aw = Z ̂ χ · dV t d λ λ · dV aw d λ ·

A common transformation of Eq. (8) yields

(9) V aw = Z ̂ χ · dV t d λ χ · dV aw d λ · λ χ V 0 + Ξ θ

which coincides with Eq. (1). The coincidence is due to the fact that dVaw/dλ<0; besides, the work hardening coefficient, θ, is given by the ratio of two structural parameters having the dimension of length, i.e. λ and X<<λ2323 Nabarro FRN. Strength of Metals and Alloys. Oxford: Pergamon Press; 1986.

24 Zaiser M, Seeger A. Long-range internal stresses, dislocation patterning and work hardening in crystal plasticity. In: Nabarro FRN, ed. Dislocations in Solids. Amsterdam: North Holland; 2002. p. 1-100.
-2525 Messerschmidt U. Dislocation Dynamics During Plastic Deformation. Berlin: Springer; 2010.; hence, θ~X/λ.

Let Eq. (4) be written as

(10) V aw = Θ λ = Θ 2 π · k ,

where ΘẐ=XVt. In view of Vaw=dλ/dT=dω/dk, we obtain =(Θ/)∙k∙dk.. Thus we obtain

(11) ω 0 ω d ω = Θ 2 π 0 k k 0 k . dk .

Hence, dispersion law of quadratic form is given as

(12) ω = ω 0 + Θ 4 π k k 0 2 .

Thus, Eq. (12) is equivalent to Eq. (2), if Θ/4πΞα.

Now we write Eq. (4) of the form

(13) λ = Z ̂ χ · V t V aw ·

By taking into account the dependence of rates Vt and Vaw on the grain size, δ55 Seeger A, Frank W. Structure Formation by Dissipative Processes in Crystals with High Defect Densities. In: Kubin LP, Martin G, eds. Non-Linear Phenomena in Materials Science. Zurich: Trans Tech Publications; 1987. p. 125-138., differentiation of Eq. (13) is performed with respect to δ as

(14) d λ d δ = Z ̂ χ · d d δ V t V aw = Z ̂ χ · V aw · dV t / d δ V t · dV aw / d δ V aw 2 ·

Transformation of Eq. (14) yields the following differential equation

(15) d λ = Z ̂ ϰ · dV t d δ · 1 V aw V t dV aw d δ · 1 V aw 2 · d δ ,

which can also be written as

(16) d λ = a 1 λ a 2 λ 2 . d δ ,

where a1=1Vt·dVtdδ=dlnVtdδ and a2=1ẐχVt·dVawdδ, since Vaw=ẐχVt·1λ. Evidently, the solution of Eq. (16) coincides with Eq. (3).

Consider also the other consequences of the invariant. Let Eq. (4) be written as

(17) χ / λ = Z ̂ V aw / V t ,

where the plastic deformation ε≈λ/X>>1. By applying the operator ∂/∂t=Dε∙∂2/∂x2 to the right and left parts of Eq. (17), consequently, we obtain

(18) ε t = Z ̂ D ε V i · 2 V aw 1 ϰ 2 + V aw 1 · 2 V t ϰ 2 ·

The ultrasound propagation rate depends weakly on the plastic deformation, ε2626 Zuev LB, Semukhin BS. Some acoustic properties of a deforming medium. Philosophical Magazine A. 2002;82(6):1183-1193.; hence, Vt≈ const. In this case, we obtain

(19) ε t = Z ̂ D ε V t 2 V aw 1 ϰ 2 + D ε 2 ε ϰ 2 ,

which is equivalent to the following differential equation for the deformation rate

(20) ε ˙ = f ε , σ + D ε ε ,

where the coefficient Dε has the dimension L2∙T-1. Equation (20) has the form of the reaction-dif fu si on equation for a concentration, ζ=φζ+Dζ˝, which is obtained when the nonlinear function, φ(ζ), is entered into the right part of Fick’s second law for diffusion ζ˙=Dζ 2727 Murray JD. Mathematical Biology - An Introduction. New York: Springer; 2002.. Equation (20) falls into the category of nonlinear relations employed for describing autowave processes, which occur in different kinds of open systems, provided that adequate variables are chosen for solving the problem 2828 Davydov VA, Davydov NV, Morozov VG, Stolyarov MN, Yamaguchi T. Autowaves in the moving excitable media. Condensed Matter Physics. 2004;7(3):565-578.,2929 Waller I, Kapral R. Spatial and temporal structure in systems of coupled nonlinear oscillators. Physical Review A. 1984;30(4):2047.. In what follows, Eq. (20) is discussed in detail.

3.4 Plastic deformation viewed as autowave generation process

By elaborating the autowave concept, we must consider the dependence of autowave patterns on the work hardening law acting at a given plastic flow stage. To make out individual flow stages on the curve σ(ε), the Lüdwick equation 3030 Pelleg J. Mechanical Properties of Materials. Dordrecht: Springer; 2012. is used

(21) σ ε = σ 0 + K ε ,

where K is a hardening modulus; σ0=const and 0≤n≤1 is a hardening exponent which varies discretely. To verify whether Eq. (21) is operative, the Kocks-Mecking method 3131 Kocks UF, Mecking H. Physics and phenomenology of strain hardening: the FCC case. Progress in Materials Science. 2003;48(3):171-273. was used for recognizing plastic flow stage. The results obtained in both cases were found to fit neatly. The in dividual work hardening stages can be distinguished on the flow curve subject to the condition that n=1nε1·1nσσ01nKconst. A total of four flow stages have been distinguished, i.e. easy glide/yield plateau, linear work hardening stage, parabolic work hardening stage and pre-failure stage. Likewise, the possible macro-locali zation patterns are limited in number: a total of four types of localized plasticity patterns are found to emerge in the deforming sample. Table 2 presents the localization patterns matched against the autowave modes. Evidently, a one-to-one correspondence exists between the autowave modes and the respective plastic flow stages (Table 2 and Fig. 5). In view of the above, the sample tested in constant-rate tension can be regarded as a universal generator of autowaves 3232 Zuev LB. Using a crystal as a universal generator of localized plastic flow autowaves. Bulletin of the Russian Academy of Sciences: Physics. 2014;78(10):957-964. that requires no maintenance of temperature or reagent concentration as is the case with, e.g. chemical reactors 66 Haken H. Information and Self-Organization. A Macroscopic Approach to Complex Systems. 3rd ed. Berlin Heidelberg: Springer-Verlag; 2006.,1919 Scott A. Nonlinear Science - Emergence and Dynamics of Coherent Structures. New Yok: Oxford University Press; 2003..

Table 2
Plastic flow stages matched against autowave modes.

Figure 5
Wave and autowave processes involved in deformation

We conclude this Section by saying that the above analysis provides a unified explanation for the autowave nature of plasticity; hence, substantial revision of traditional notions in this field is required. Now that the work hardening process is regarded as evolution of the autowave modes, deformation kinetics analysis must involve different principles so as to formulate a new viewpoint of the nature of multi-stage plastic flow. The autowave plastic deformation exhibits regular features, which are consequences of Eq. (4); all the empirical coefficients in Eqs. (1) - (3) have been assigned a physical meaning. In the frame of this concept the micro-scale level is related to the macro-scale features of localized plastic deformation by Eq. (4), which should be regarded as 'master equation' of the plasticity theory being developed.

4. The two-component model of plastic flow

4.1 Nonlinear equations for localized plastic flow

In general, the processes involved in self-organization are conventionally regarded as an interplay of an activator and a damper 66 Haken H. Information and Self-Organization. A Macroscopic Approach to Complex Systems. 3rd ed. Berlin Heidelberg: Springer-Verlag; 2006.,2828 Davydov VA, Davydov NV, Morozov VG, Stolyarov MN, Yamaguchi T. Autowaves in the moving excitable media. Condensed Matter Physics. 2004;7(3):565-578.. An understanding of how the both factors relate to the localized plastic flow could illuminate the roles they play. It is therefore assumed that the plastic deformation, ε, is an activator and the elastic stresses, σ, a damper.

It would be reasonable to describe the kinetics of the activator using Eq. (20), which was inferred as a consequence of invariant (4). In turn, the stress relaxation kinetics can be described using the Euler equation for viscous liquid flux 3333 Landau LD, Lifshitz EM. Fluid Mechanics. 2nd ed. Oxford: Pergamon Press; 1987., which has the form

(22) t pv i = x k ik ,

where ik=pδik+pvivkσvis=σikpvivk is momentum flux density tensor; δik, unit tensor; p, pressure; νi and νk, flux velocity components. The stress tensor σik=-pδikvis is the sum of elastic and viscous stresses, respectively, i.e. σel=-pδik and σvis. In the case of plastically deforming medium, σ=σelvis, i.e. σ˙=σ˙el+σ˙vis· It is reported in 3131 Kocks UF, Mecking H. Physics and phenomenology of strain hardening: the FCC case. Progress in Materials Science. 2003;48(3):171-273.,3434 V.I. Al'shits, V.L. Indenbom, Dinamika dislokatsii. In: Nabarro FRN, ed. Dislocations in Solids. Amsterdam: New Holland; 1986. that σ˙elgσ,ε=Mpmb2σ/B=MpmbVdislVdisl (here M is elastic modulus for the sys tem 'sample - testing machine'; ρm is mobile dislocation density and Vdisl is dislocation motion rate).

Due to the inhomogeneous inter nal elastic strain field, viscous stresses, σvis, will form in the deforming medium. The viscous stresses are re la ted to the variations in the elastic wave rate which are linear with respect to stresses, i.e. Vt=Vt0+κσ2626 Zuev LB, Semukhin BS. Some acoustic properties of a deforming medium. Philosophical Magazine A. 2002;82(6):1183-1193.. Here Vt0 is the transverse elastic wave rate in the absence of stres ses and κ=const. Assuming that σvis=B∂Vt/∂x (here B is medium’s dynamic viscosity), we can write ∂σvis/∂t=Vt∂/∂x (B∂Vt/∂x)= BVt2Vt/∂x2. Hence, the relaxation rate is given for viscous stres ses as ∂σvis/∂t = BVt2Vt/∂x2 = BκVt2σ/∂x2. Apparently,

(23) σ / t = g ε , σ + D σ 2 σ / x 2 ,

where Dσ=BκVt is a transport coefficient having the dimension L2∙T-1. Thus, Eq. (23) can be used to describe the damper kinetics in the deforming medium by virtue of the fact that Dσ≡Ddamp. The right part of Eq. (23) is the sum of relaxation rates of elastic and viscous stresses, σ˙e=g(ε,σ) and σ˙vis=Dσ∙∂2σ/∂x2, respectively. The nonlinear function g(ε,σ) accounts for the elastic stress redistribution among neighboring material micro-volumes ahead of the moving plastic deformation front and the diffusion-like term Dσ∙∂2σ/∂x2 is responsible for elastic stress redistribution among material volumes via macro-scale stochastic processes.

The above line of mathematical reasoning can be made more accessible by suggesting that the flow rates ε˙ and σ˙ incorporate both the 'hydrodynamic' and 'diffusion' com ponents. The hydrodynamic components are given by the nonlinear functions f(ε,σ)~Vdisl and g(σ,ε)~Vdisl from Eqs. (20) and (23), correspondingly. These have to do with the steady moti on of deformation fronts along the sample, with the local stress concentrators occurring on the fronts being activated one by one. The diffusion components are given by the terms Dε2ε/∂x2 and Dσ2σ/∂x2 from Eqs. (20) and (23). These are responsible for the deformation initiated in material volumes at macroscopic distance from the active deformation front.

Thus, the resultant system of equations

ε ˙ = f ε , σ + D ε ε σ ˙ = g ε , σ + D σ σ 24 a 24 b

may be used for autowave mode analysis, provided that the nonlinear functions f(ε,σ) and g(σ,ε) in explicit form are available. Equations (20), (23), a system of Eq. (24a, b) and the reasoning involved in the derivation thereof served the basis for the development of two component model of plasticity. Two versions of the same model are discussed below.

4.2 The two-component model. The autowave version

Note that the coefficients Dε and Dσ from the system of Eqs. (24a) and (24b) have dimensions L2∙T-1, which coincide with those of the products λ∙Vaw and X∙Vt from invariant (4). Hence,

(25a) λ · V aw D ε

and

(25b) χ · V t D σ ·

The above suggests that invariant (4) is equivalent to the ratio Dε/Dσ=2/3<1, i.e. Dσ ≡ Ddamp > Dε ≡ Dactiv. The condition Ddamp>Dactiv is a prerequisite for auto wave ge ne ration in the active medium 66 Haken H. Information and Self-Organization. A Macroscopic Approach to Complex Systems. 3rd ed. Berlin Heidelberg: Springer-Verlag; 2006.. The autowave structure formation should be regarded as a basic attribute of the self-organizing active medium 66 Haken H. Information and Self-Organization. A Macroscopic Approach to Complex Systems. 3rd ed. Berlin Heidelberg: Springer-Verlag; 2006.. In a general case, the likelihood that self-organization processes will be initiated in the active medium depends on whether the medium itself is capable of separating spontaneously into information and dynamic subsystems 3535 Kadomtsev BB. Dynamics and information. Physics-Uspekhi. 1994;37(5):425.. The main features of plastic flow might be explained by assuming that the information subsystem is related to acoustic emission pulses generated by dislocation shears and the dynamic subsystem, to shears proper 3636 Zuev LB, Barannikova SA. Experimental study of plastic flow macro-scale localization process: Pattern, propagation rate, dispersion. International Journal of Mechanical Sciences. 2014;88:1-7.. The evolution of two subsystems is described by Eqs. (20) and (23).

Based on the assumptions above, a two-component model of plastic flow is proposed which operates in accordance with the scheme presented in Fig. 6. Due to the stress concentrator decay (1), stress relaxation will occur which causes generation of acoustic emission pulses. The stress relaxation results in the liberation of energy which is absorbed by the remaining stress concentrators which act as energy-sink (2). This phenomenon is known as acoustic-plas tic effect 3737 Burnett JK, ed. Theory and Uses of Acoustic Emission. New York: Nova Science Publishers; 2012.. As new stress relaxation acts are initiated, shear processes will continue to occur in the dynamic subsystem, generating thereby a series of acoustic pulses. Thus the basic idea of the model being developed is that the acoustic emission and the acoustic-plastic effect are in no way interdependent. This issue has been neglected thus far. In support of this interpretation one can argue that the elastic-plastic invariant is given by Eq. (5), which contains the term ξ1=Vt ρ for medium's acoustic resistance.

Figure 6
A schematic of the generation of localized plasticity fronts dislocation shears (stress concentrators); ⚋⚋⚋ shears due to decay of stress concentrators; ⚋⚋⚋⚋⚋⚋⚋⚋🠊 elastic pulse trajectory

To verify the model’s validity, the expectation times, τ* and τ**, are estimated for the thermally activated relaxation acts 3838 Caillard D, Martin JL, eds. Thermally Activated Mechanisms in Crystal Plasticity. Volume 8. Oxford: Pergamon; 2003.. In the event that the external stress alone is operating,

(26) t * = ω D 1 exp U 0 γ σ k B T ;

in the event that both the external stress and the acoustic pulse are operating,

(27) t * * ω D 1 exp U 0 γ σ U ac k B T = ω D 1 exp U 0 γ σ + ε ac E k B T ·

In Eqs. (26) and (27) the activation enthalpy, U0-γσ≈0.5 eV3838 Caillard D, Martin JL, eds. Thermally Activated Mechanisms in Crystal Plasticity. Volume 8. Oxford: Pergamon; 2003.. Due the action of acoustic pulse having amplitude, εac≈ 2∙10-6, reduction in the activation enthalpy is ΔUac ≈ γεacE ≈ 0.1 eV and kBT≈ 1/40 eV. Under the above conditions, τ* ≈5∙10-5 s and τ** ≈9∙10-7 s << τ*. The estima te, rough as it is, evidently speaks for the proposed model. It is thus proved that the events occurring in the acoustic (information) and dislocation (dynamic) subsystems are interrelated.

The effect of transverse ultrasound wave splitting in the field of elastic stresses can be used to estimate the autowave length 3939 Tokuoka T, Iwashizu Y. Acoustical birefringence of ultrasonic waves in deformed isotropic elastic materials. International Journal of Solids and Structures. 1986;4(3):383-389.. Assume that a transverse ultrasound pulse is emitted by an elementary shear. The maximal power in the acoustic emission spectrum corresponds to the frequency, ωa ≈ 106 Hz 3737 Burnett JK, ed. Theory and Uses of Acoustic Emission. New York: Nova Science Publishers; 2012.. Due to the pulse splitting occurring in an elastically stressed area, two orthogonal polarized waves will form; these have lengths ς11a and ς22a and propagation rates ν1≠ν2. A difference in the wavelengths is given in 3939 Tokuoka T, Iwashizu Y. Acoustical birefringence of ultrasonic waves in deformed isotropic elastic materials. International Journal of Solids and Structures. 1986;4(3):383-389. as

(28) δ ς = ς 2 ς 1 = v 2 v 1 ω a = σ 2 σ 1 2 ω a pV t ·

An estimate of the same values can be obtained by assuming that a difference in principal normal stresses, σ2-σ1≈ 108 Pa; material density, ρ≈ 5∙103 kg/m3 and sound rate, Vt≈3∙103 m/s. Using this line of reasoning, we obtain that δς≈ 10-4m. This rough estimate suggests that the maximal energy of the elastic wave is accumulated at distance ~ς2/δς≈ 10-2m ~λ from the pul se origin. This is a plausible explanation for the fact that the new localized plasticity front emerges at distance ~λ from the existing deformation front.

4.3 The two-component model. The quasi-particle version

The above numerical analysis demonstrates that the products λ∙Vaw∙ρ∙X3 obtained for fourteen metals are close to the quantum Planck constant h = 6.626∙10-34 J∙s 4040 Landau LD, Lifshitz EM. Quantum Mechanics (Non-relativistic Theory). London: Butterworth-Heinemann; 1977.. On the strength of da ta presented in Table 3, we write

Table 3
Planck constant values, h, and autolocalizon masses, ma-l, calculated for studied metals.

(29) λ 1 · V aw , i · ρ i · χ i 3 = h i ,

where 1≤i≤14. The average value 〈h〉 (6.95±0.48)∙10-34 J∙s; hence, the ratio 〈h〉/h=1.05±0.07≈1. Without doubt, this intriguing result requires statistical verification. To decide whether the values 〈h〉 and h are equal or different, they were compared with the help of Student's t̂-criterion 4141 Hudson DJ. Statistics. Lectures on Elementary Statistics and Probability. Geneva: CERN; 1964., which was calculated from the formula

(30) t ̂ = h h σ ̂ 2 · n 1 · n 2 n 1 + n 2 ,

where n1 14 is the number of estimates of hi from Eq. (32) and n2=1. This suggests that high-accuracy measurements were performed in the absence of dispersion. The estimate of ove rall dispersion, σ̂2, can be made for the quantities 〈h〉 and h4141 Hudson DJ. Statistics. Lectures on Elementary Statistics and Probability. Geneva: CERN; 1964. as

(31) σ ̂ 2 = i = 1 n 1 hi h 2 + 1 1 h h 2 n 1 + n 2 2 = i = 1 n 1 hi i h 2 . n 1 + n 2 2

The calculation of the t̂-criterion demonstrates that the values 〈h〉 and h really belong to the sampling from one and the same general population with the probability higher than 95%. Thus, Eq. (29) actually determines the Planck constant. This leads us to believe that quantum mechanics prin ciples are also suitable for investigations performed in the frame of plastic deformation physics.

This finding led us to believe that a hypothetical a quasi-particle might be introduced for addressing the localized plasticity autowave. This procedure is conventionally applied in solids physics 4242 Madelung O. Introduction to Solid-State Theory. Berlin: Springer Science; 1996.. By omitting the index 'i' from Eq. (29), we obtain

(32) ρ · χ 3 = ρ Ω = m ef = h / λ V aw ,

which is easily identified with the well-known de Broglie equation, which gives the effective mass of a quasi-particle moving with velocity Vaw as mef≈ ρX34343 Billingsley JP. The possible influence of the de Broglie momentum-wavelength relation on plastic strain "autowave" phenomena in "active materials". International Journal of Solids and Structures. 2001;38(24-25):4221-4234.. Thus, a quasi-particle is postulated which corresponds to the localized plasticity autowave; its effective mass is given as ma-l=h/λVaw. The hypothetical quazi-particle has been called 'autolocalizon'4444 Zuev LB. The linear work hardening stage and de Broglie equation for autowaves of localized plasticity. International Journal of Solids and Structures. 2005;42(3-4):943-949.,4545 Barannikova SA, Ponomareva AV, Zuev LB, Vekilov YK, Abrikosov IA. Significant correlation between macroscopic and microscopic parameters for the description of localized plastic flow auto-waves in deforming alloys. Solid State Communications. 2012;152(9):784-787.. Using Eq. (32), the average mass of the autolocalizon was calculated for fourteen me tals; the value obtained, 〈ma-l〉= 1.7±0.2 a.m.u. An attempt of similar kind is worthy of notice. Thus the authors in 4646 Morozov EM, Fridman YB. Trajectories of the brittle-fracture cracks as a geodesic lines on the surface of a body. Soviet Physics - Doklady. 1962;6(7):619-621. introduced a quasi-particle, so-called 'crackon', which was identified with the tip of growing brittle crack. It was also attempted to introduce so-called 'frustron', which might be appropriate for descriptions of the initial stage of lattice defect generation 4747 Olemskoi AI. Theory of Structure Transformations in Non-Equilibrium Condensed Matter. New York: Nova Science Publishers; 1999..

A striking analogy can be drawn between the auto localizons and the 'rotons'. The latter quasi-particles were introduced in the theory of liquid He4 super fluidity 4848 Landau LD, Lifshitz EM. Statistical Physics. London: Butterworth-Heinemann; 1980.. The auto localizon and the ro ton have a dispersion law of quadratic form; the effective mass of roton, mrot≈0.64 a.m.u. 4848 Landau LD, Lifshitz EM. Statistical Physics. London: Butterworth-Heinemann; 1980., is close to that of auto localizon. In view of the above, the given approach could be elaborated in more detail.

Let Eq. (29) be written as

(33) λ V aw ρ = h / χ 3 ,

where both terms have the dimension of dynamic viscosity, i.e. M∙L-1∙T-1≡Pa∙s. Using Eq. (33), calculations were performed for all studied metals; the resultant value, λVawρ=h/X3≈5∙10-4 Pa∙s. The latter value is close to the coefficient of dislocation drag, В, obtained for quasi-viscous dislocation motion rate Vdisl≈(bσ)/B 3434 V.I. Al'shits, V.L. Indenbom, Dinamika dislokatsii. In: Nabarro FRN, ed. Dislocations in Solids. Amsterdam: New Holland; 1986.. It is thus concluded that elastic-plastic invariant (4) might be employed in the frame of alternative approach. In view of the equality

(34) λ V aw = h / p · χ 3 = h / m a 1 ,

we may write, analogously,

(35) χ V t = h / m ph ,

where mph is taken to be phonon mass. Now invariant (4) may be written as

(36) Z ̂ · h λ V aw = h χ V t ,

which reduces to the balance of masses as 2ma-l=3mph, i.e. three phonons would produce a pair of autolocalizons. This suggestion undoubtedly requires verification. It might be well to point out that si milar complex processes occurring in the phonon gas were described earlier 4949 Srivastava GP. The Physics of Phonons. New York: Taylor and Francis; 1990.,5050 Umezava H, Matsumoto H, Tachiki M. Thermo Field Dynamics and Condensed States. Amsterdam: North-Holland; 1982..

In the frame of quasi-particle approach the deforming medium might be viewed as a mixture of phonons and autolocalizons. It is thus suggested that the random walk of the Brownian particle is 4848 Landau LD, Lifshitz EM. Statistical Physics. London: Butterworth-Heinemann; 1980.

(37) S K B T π Br a 1 t ,

where the time, τ=2π/ω≈103 s; the dynamic viscosity of the phonon gas, B≈5∙10-4 Pa∙s (see above) and kBT 1/40 eV for T=300 K. Hence, the effective size of autolocalizon, ralΩ3χ1010 m and the quasi-particle walk, S≈10-2 m≈λ, which agrees with both the experimental value and that calculated from Eq. (28). By rewriting Eq. (37) as

(38) S 2 t k B T π Br a 1 ,

we obtain S2/τ≈Dε≈1.3∙10-7 m2/s. The above suggests that the processes involved in the plastic flow can be addressed effectively in the frame of quasi-particle and auto wave approaches.

5. Localized plasticity autowaves and dislocation theory

5.1 The autowave deformation and the Taylor-Orowan equation

The problem this approach seeks to resolve is this: little is known about its relation to the dislocation theory which serves as the basis for the overwhelming majority of traditional models in plasticity physics 2323 Nabarro FRN. Strength of Metals and Alloys. Oxford: Pergamon Press; 1986.

24 Zaiser M, Seeger A. Long-range internal stresses, dislocation patterning and work hardening in crystal plasticity. In: Nabarro FRN, ed. Dislocations in Solids. Amsterdam: North Holland; 2002. p. 1-100.
-2525 Messerschmidt U. Dislocation Dynamics During Plastic Deformation. Berlin: Springer; 2010.,5151 Friedel J. Dislocations. Oxford: Pergamon Press; 1964.,5252 Kuhlmann-Wilsdorf D. The LES theory of solid plasticity. In: Nabarro FRN, Duesbery MS, eds. Dislocations in Solids. Amsterdam: New Holland; 2002. p. 211-342.. Therefore, it is absolutely necessary to relate of the autowave equations derived herein to the dislocation mechanisms of plasticity. Note that the idea about quantization of dislocation deformation is in no way objectionable, since the Burgers vector, b=a1+a2+a3, is usually considered as 'a quantum of shear deformation' and its components, ai, are topological quantum numbers 5050 Umezava H, Matsumoto H, Tachiki M. Thermo Field Dynamics and Condensed States. Amsterdam: North-Holland; 1982.,5353 Kadic A, Edelen DGB. A Gauge Theory of Dislocations and Disclinations. Berlin Heidelberg: Springer-Verlag; 1983.. Now consider the function fε,σ=ε·Dε in Eq. (20). For a homogeneous distribution of dislocations with average spacing d, ε'≈d-1∙ (b/d)≈b∙d-2m (here b/d is shear per dislocation and d-2≈ρm is mobile dislocation density). Given Dε≈L∙Vdisl (here L≈αx is dislocation path and Vdisl=const, dislocation rate), we obtain D'ε=αVdisl. Hence, Eq. (20) reduces to the equality

(39) ε ˙ = α b ρ m V disl + D ε ε ,

where the first term from the right side coincides with the Taylor-Orowan equation for dislocation deformation, i.e. ε˙=bρmVdisl, which might be considered now as a special case of Eq. (39). However, Eq. (39) is applicable to more general cases, e.g. media having high dislocation density, provided the diffusion-like term Dεε" is added to the right side of the Taylor-Orowan equation. To clarify this purely formal procedure, we shall give some explanation of the condition to be met. Given ε˙=const by constant-rate tensile loading, the required level of dislocation flux, ρmVdisl, has to be maintained. If the condition is not met, owing to, e.g. a decrease in mobile dislocation density, the medium will initiate deformation processes in front of the plasticity nucleus remote from the nuclei already in existence - otherwise sample fracture will occur. This representation provides a new way of tackling nonlinear problems connected with the nature and evolution of dislocation substructures 2424 Zaiser M, Seeger A. Long-range internal stresses, dislocation patterning and work hardening in crystal plasticity. In: Nabarro FRN, ed. Dislocations in Solids. Amsterdam: North Holland; 2002. p. 1-100.,2525 Messerschmidt U. Dislocation Dynamics During Plastic Deformation. Berlin: Springer; 2010.,5252 Kuhlmann-Wilsdorf D. The LES theory of solid plasticity. In: Nabarro FRN, Duesbery MS, eds. Dislocations in Solids. Amsterdam: New Holland; 2002. p. 211-342..

5.2 Localized plasticity autowaves and work hardening coefficient

A number of well-established models link work hardening processes to the long- or short-range interaction of dislocations 5151 Friedel J. Dislocations. Oxford: Pergamon Press; 1964.,5252 Kuhlmann-Wilsdorf D. The LES theory of solid plasticity. In: Nabarro FRN, Duesbery MS, eds. Dislocations in Solids. Amsterdam: New Holland; 2002. p. 211-342.. In what follows, the autowave mechanism has to be related to the work hardening phenomena in terms of plasticity physics. Assume that the work hardening coefficient is given as θ≈W/Q2323 Nabarro FRN. Strength of Metals and Alloys. Oxford: Pergamon Press; 1986. (here W≈Eb2ρs is the energy stored by plastic defor ma tion; ρs, immobile dislocation density; Q≈σbLdρm, energy dissipated by mobile dislocati ons having density, ρm, and path, Ld). Now it can be written

(40) θ Eb 2 ρ s σ bL d ρ m b ε e L d · ρ s ρ m ,

where εe=σ/E; Ld = Λ∙(ε-ε*)-1; Λ depends on the kind of material 2424 Zaiser M, Seeger A. Long-range internal stresses, dislocation patterning and work hardening in crystal plasticity. In: Nabarro FRN, ed. Dislocations in Solids. Amsterdam: North Holland; 2002. p. 1-100. аnd ε* is the strain for the onset of linear work hardening stage. It follows from Eqs. (1) and (40) that

(41) V aw Ξ · Λ b · ε ε * ε e · ρ m ρ s ·

With growing density of immobile defects, ρs, the value Vaw will grow less. With increasing amo unt of energy dissipated to he at, the deforming medium would warm up, which greatly increases the likelihood of thermally activated plastic deformation and of autowave rate growth.

Now let dVaw∼Ld; hence, we obtain 2424 Zaiser M, Seeger A. Long-range internal stresses, dislocation patterning and work hardening in crystal plasticity. In: Nabarro FRN, ed. Dislocations in Solids. Amsterdam: North Holland; 2002. p. 1-100.,2525 Messerschmidt U. Dislocation Dynamics During Plastic Deformation. Berlin: Springer; 2010.

(42) θ zb / 3 ,

where z is the number of dislocations in a planar pileup. It follows from the above that dVaw∼Ld∼Λ∼θ-2. The data obtained for a range of materials suggest that ε-ε*≈const2424 Zaiser M, Seeger A. Long-range internal stresses, dislocation patterning and work hardening in crystal plasticity. In: Nabarro FRN, ed. Dislocations in Solids. Amsterdam: North Holland; 2002. p. 1-100.; however, the value θ is found to vary for different materials, i.e. dθ≠0. Then we can write

(43) dV aw zb ε ε * 1 θ 2 d θ .

Integration of Eq. (43) yields Vaw∼θ-1. Finally, a special case of Eq. (1) is written as

(44) V aw = V 0 * + J / θ * ,

where θ*=dσ/dε is a dimension characteristic of the plastic flow process (see above). The values calculated for alloyed single γ-Fe crystals are as follows: V0*2.1·105 m/s and J≈3.4∙104 Pa∙m/s. Let J≈σVm (here σ is flow stress and Vm is mobile grip rate). Since Pa∙m/s=W∙m-2, the quantity J acquires the mea ning of flux power from the loading machine through the sample. Given σ≤103 MPa and Vm=3.3∙10-6 m/s, we obtain J≤3.3∙104 W∙m-25454 Zuev LB, Danilov VI. Plastic deformation modelled as a self-excited wave process at the meso- and macro-level. Theoretical and Applied Frature Mechanics. 1998;30(3):175-184.

55 Zuev LB, Danilov VI. A self-excited wave model of plastic deformation in solids. Philosophical Magazine A. 1999;79(1):43-57.
-5656 Zuev LB, Danilov VI, Barannikova AS, Zykov IY. A new type of plastic deformation waves in solids. Applied Physics A. 2000;71(1):91-94..

Thus the work hardening process is addressed above in the frame of conventional dislocation model by assuming that a changeover in the work hardening stages is due to variation in the distribution of stress concentrators 5151 Friedel J. Dislocations. Oxford: Pergamon Press; 1964.. Hence, the same factor might be responsible for the generation of new autowave modes in the active medium.

6. Conclusions

Solids plasticity is addressed above in the frame of autowave concept. The given approach might fall far short of a completely theoretical prediction. In point of fact, it might be regarded as an attempt at envision of the complexities of the plastic flow process, which would enable formulation of contemporary views of this phenomenon. Hopefully, more rigorous techniques would be developed for tackling the problem of plasticity. Thus far we have the pleasure of bringing to your notice the following conclusions.

  1. The localization behavior of plastic deformation has been studied for all the plastic flow stages. Localized plasticity patterns are found to emerge in the deforming medium. A total of four pat tern kinds have been recognized in studied materials. It is found that the kind of pattern observed for the given flow stage strictly corresponds to the work hardening mechanism involved in the deformation.

  2. The kinetics of plastic deformation and stresses is described using autowave equations derived on the base of continuum media mechanics.

  3. On the base of experimental data elastic-plastic deformation invariant is obtained, which is a master equation for plasticity mechanics. In the frame of autowave model the invariant serves to relate the characteristics of localized plasticity autowaves to those of elastic waves. The distinctive features of localized plasticity autowaves are described by the consequences from the invariant.

  4. A two-component model of localized plasticity is proposed which is based on the assumption that shear processes interact with acoustic pulses. The autowave model is complemented by the quasi-particle model; the both versions are of equivalent status.

  5. A relationships are established between the autowave representations and certain conventional dislocation models, which precludes any controversy between the proposed auto wave approach and the existing work hardening theories.

7. Acknowledgements

The work was performed within the Program of Fundamen-tal Research of State Academies of Sciences for the period of 2013–2020 and was supported by Tomsk State University in the framework of the Competitiveness Improvement Program.

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    Zuev LB. The linear work hardening stage and de Broglie equation for autowaves of localized plasticity. International Journal of Solids and Structures 2005;42(3-4):943-949.
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    Barannikova SA, Ponomareva AV, Zuev LB, Vekilov YK, Abrikosov IA. Significant correlation between macroscopic and microscopic parameters for the description of localized plastic flow auto-waves in deforming alloys. Solid State Communications 2012;152(9):784-787.
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    Zuev LB, Danilov VI. Plastic deformation modelled as a self-excited wave process at the meso- and macro-level. Theoretical and Applied Frature Mechanics 1998;30(3):175-184.
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    Zuev LB, Danilov VI. A self-excited wave model of plastic deformation in solids. Philosophical Magazine A 1999;79(1):43-57.
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Publication Dates

  • Publication in this collection
    08 Aug 2019
  • Date of issue
    2019

History

  • Received
    28 Oct 2018
  • Reviewed
    08 May 2019
  • Accepted
    21 May 2019
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